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Publication
ID31453994Published Date2019-09-21JournalDalton transactions (Cambridge, England : 2003), 2019-09-21, Volume 48
While the loading of liquid or solid materials in the pores of metal-organic frameworks (MOFs) can yield composite materials with novel and useful emergent properties, the loading of solids, and ionic solids in particular, can be challenging. We report the loading of the salts NHNO and LiNO in the MOF UiO-66. The relatively low-melting NHNO is loaded in UiO-66 in a solvent-free method, and loading is complete in 8 h at 75 °C, far below the melting point of NHNO. The higher-melting LiNO requir…
Publication
ID31453609Published Date2019-09-21JournalChemical communications (Cambridge, England), 2019-09-21, Volume 55
A highly reducing diquat-type molecule was explored as a negative electrolyte for nonaqueous redox flow batteries. The molecule displays a highly negative 2/0 reduction potential of -1.67 V (vs. ferrocene), a low mass per electron transferred, and good solubility in CHCN in both redox states. Moderate capacity retention is observed during electrochemical charge-discharge cycling. A pathway for decomposition during electrochemical cycling is elucidated, and this provides a clear path forward f…
Publication
ID31326119Published Date2019-09-20JournalJournal of biomechanics, 2019-09-20, Volume 94
Severity of aortic coarctation (CoA) is currently assessed by estimating trans-coarctation pressure drops through cardiac catheterization or echocardiography. In principle, more detailed information could be obtained non-invasively based on space- and time-resolved magnetic resonance imaging (4D flow) data. Yet the limitations of this imaging technique require testing the accuracy of 4D flow-derived hemodynamic quantities against other methodologies. With the objective of assessing the feasib…
Simone Saitta Selene Pirola Filippo Piatti Emiliano Votta Federico Lucherinishow 8 more
Imperial College LondonImperial College LondonPolitecnico di MilanoPolitecnico di MilanoUniversity of MichiganUniversity of Michigan
Publication
ID31506041Published Date2019-09-27JournalJournal of the Royal Society, Interface, 2019-09-27, Volume 16
The unfolded protein response (UPR) is a collection of cellular feedback mechanisms that seek to maintain protein folding homeostasis in the endoplasmic reticulum (ER). When the ER is 'stressed', through either high protein folding demand or undersupply of chaperones and foldases, stress sensing proteins in the ER membrane initiate the UPR. Recently, experiments have indicated that these signalling molecules detect stress by being both sequestered by free chaperones and activated by free unfo…
Publication
ID31480937Published Date2019-09-27JournalBiology letters, 2019-09-27, Volume 15
Anthropogenic environmental change is predicted to disrupt multitrophic interactions, which may have drastic consequences for population-level processes. Here, we investigate how a large-scale human-mediated disturbance affects the abundance of North America's most venomous caterpillar species, Megalopyge opercularis. Specifically, we used a natural experiment where netting was deployed to cover the entire canopies of a subset of mature southern live oak trees (Quercus virginiana) to exclude …
Glen R Hood Mattheau Comerford Amanda K Weaver Patricia M Morton Scott P Egan
Wayne State UniversityWayne State UniversityRice UniversityRice University
Publication
ID31385588Published Date2019-09-29JournalHuman reproduction (Oxford, England), 2019-09-29, Volume 34
Is there an association between air pollution exposures and the risk of spontaneous abortion (SAB)?Higher exposure to particulate matter (PM) air pollution above and beyond a woman's average exposure may be associated with greater risk of SAB, particularly among women experiencing at least one SAB during follow-up.There is sufficient biologic plausibility to suggest that air pollution adversely affects early pregnancy outcomes, particularly pregnancy loss; however, the evidence is limited.Our…
Audrey J Gaskins Jaime E Hart Jorge E Chavarro Stacey Missmer Janet W Rich-Edwardsshow 2 more
Harvard T.H. Chan School of Public HealthHarvard T.H. Chan School of Public HealthHarvard UniversityHarvard UniversityBrigham and Women's HospitalBrigham and Women's HospitalPartners HealthCarePartners HealthCareMichigan State UniversityMichigan State Universityshow 1 more
Publication
ID31331642Published Date2019-09-17JournalBiochemical and biophysical research communications, 2019-09-17, Volume 517
Interleukin-6 (IL-6) has become a target of interest for drug development aiming to treat diabetic retinopathy. Since IL-6 signaling can promote beneficial as well as detrimental effects via two different signaling pathways, the objective of the present study was to investigate the effects of classical IL-6 and IL-6 trans-signaling on human Müller cells (HMC), which are important for the development of diabetic retinopathy. HMCs were cultured in normal (5 mmol/L) and high (25 mmol/L) glucose …
Publication
ID31432810Published Date2019-09-16JournalChemical communications (Cambridge, England), 2019-09-16, Volume 55
New chelating bis(alkoxide) ligand H[OO] and its iron(ii) complex Fe[OO](THF) are described. The coordination of the ligand to the metal center is reminiscent of the coordination of two monodentate alkoxides in previously reported Fe(OR)(THF) species. Fe[OO](THF) catalyzes selective and efficient dimerization of non-bulky aryl nitrenes to yield the corresponding azoarenes.
Publication
ID31352879Published Date2019-09-16JournalPhilosophical transactions of the Royal Society of London. Series B, Biological sciences, 2019-09-16, Volume 374
Mammalian carnivores are declining worldwide owing to human activities. Behavioural indicators have the potential to help identify population trends and inform conservation actions, although this area of research is understudied. We investigate whether behaviour is linked to abundance in a community of carnivores in the Masai Mara National Reserve, Kenya. Anthropogenic disturbance increased exponentially in parts of the Reserve between 1988 and 2017, mainly owing to daily incursions by large …
Publication
ID31233711Published Date2019-09-15JournalAnalytical biochemistry, 2019-09-15, Volume 581
A previous approach was established that allowed direct identification of pyridoxal-5'-phosphate (PLP) bonding sites in proteins using mass spectrometry after tryptic proteolysis. The approach required peptide mass fingerprinting owing to suppressed amide backbone fragmentation in favor of side-chain elimination of diagnostic product ions from PLP-derivatized lysyl residues. While sufficient for purified proteins, unambiguous sequence determination is needed to assign PLP bonding sites in unk…
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